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Performance and degradation of Proton Exchange Membrane Fuel Cells: State of the art in modeling from atomistic to system scale

  • Proton Exchange Membrane Fuel Cells (PEMFC) are energy efficient and environmentally friendly alternatives to conventional energy conversion systems in many yet emerging applications. In order to enable prediction of their performance and durability, it is crucial to gain a deeper understanding of the relevant operation phenomena, e.g., electrochemistry, transport phenomena, thermodynamics as wellProton Exchange Membrane Fuel Cells (PEMFC) are energy efficient and environmentally friendly alternatives to conventional energy conversion systems in many yet emerging applications. In order to enable prediction of their performance and durability, it is crucial to gain a deeper understanding of the relevant operation phenomena, e.g., electrochemistry, transport phenomena, thermodynamics as well as the mechanisms leading to the degradation of cell components. Achieving the goal of providing predictive tools to model PEMFC performance, durability and degradation is a challenging task requiring the development of detailed and realistic models reaching from the atomic/molecular scale over the meso scale of structures and materials up to components, stack and system level. In addition an appropriate way of coupling the different scales is required. This review provides a comprehensive overview of the state of the art in modeling of PEMFC, covering all relevant scales from atomistic up to system level as well as the coupling between these scales. Furthermore, it focuses on the modeling of PEMFC degradation mechanisms and on the coupling between performance and degradation models.show moreshow less

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Metadaten
Document Type:Article (reviewed)
Zitierlink: https://opus.hs-offenburg.de/2216
Bibliografische Angaben
Title (English):Performance and degradation of Proton Exchange Membrane Fuel Cells: State of the art in modeling from atomistic to system scale
Author:Thomas Jahnke, Georg Futter, Arnulf Latz, Thomas Malkow, Georgios Papakonstantinou, Georgios Tschotridis, Pascal Schott, Mathias Gérard, Manuelle Quinaud, Matias Quiroga, Alejandro A. Franco, Kourosh Malek, Frederico Calle-Valejo, Rodrigo Ferreira de Morais, Torsten Kerber, Philippe Sautet, David Loffreda, Stephan Strahl, Maria Serra, Pierpaolo Polverino, Cesare Pianese, Manik MayurStaff MemberORCiD, Wolfgang G. BesslerStaff MemberORCiDGND, Costis Kompis
Year of Publication:2016
Publisher:Elsevier
First Page:207
Last Page:233
Parent Title (English):Journal of Power Sources
Volume:304
ISSN:0378-7753
DOI:https://doi.org/10.1016/j.jpowsour.2015.11.041
Language:English
Inhaltliche Informationen
Institutes:Forschung / INES - Institut für nachhaltige Energiesysteme (bis 18.11.2021: Institut für Energiesystemtechnik)
Fakultät Elektrotechnik und Informationstechnik (E+I) (bis 03/2019)
Institutes:Bibliografie
GND Keyword:Brennstoffzelle
Formale Angaben
Open Access: Closed Access 
Licence (German):License LogoUrheberrechtlich geschützt